Journal
DALTON TRANSACTIONS
Volume 45, Issue 43, Pages 17290-17295Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6dt03160a
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Funding
- Fundamental Research Funds for the Central Universities [WK3450000001, WK2060200012]
- CAS Youth Innovation Promotion Association
- National Natural Science Foundation of China [21274139, 21674106]
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A novel bistalkynylplatinum(II)] terpyridine molecular tweezer with conformationally-rigid spacer has been designed and synthesized, which shows enhanced binding affinity towards the complementary guests when compared to its semi-rigid counterpart. Moreover, a three-component supramolecular recognition system comprised of the molecular tweezer and two electron-rich guests was established. Reversible switching of the host-guest binding preference can be achieved via adding a trace amount of hexafluoroisopropanol (HFIP) into chloroform. Such a system will be interesting for the future construction of intelligent molecular machines and devices.
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