4.7 Article

Deep learning for classification of time series spectral images using combined multi-temporal and spectral features

Journal

ANALYTICA CHIMICA ACTA
Volume 1143, Issue -, Pages 9-20

Publisher

ELSEVIER
DOI: 10.1016/j.aca.2020.11.018

Keywords

Spectral imaging; Chemometrics; Long short-term memory; Time series; Classification

Funding

  1. European Research Council (ERC) [335508-BioWater]
  2. Science Foundation Ireland (SFI)

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This study proposes a hybrid approach of PCA and deep learning for time series spectral imaging datasets, achieving substantial improvement in pixel-wise classification accuracy and perfect object-based classification accuracy. The method is powerful in utilizing time dependencies and adaptable to non-congruent images over time sequences and spectroscopic data.
Time series spectral imaging facilitates a comprehensive understanding of the underlying dynamics of multi-component systems and processes. Most existing classification strategies focus exclusively on the spectral features and they tend to fail when spectra between classes closely resemble each other. This work proposes a hybrid approach of principal component analysis (PCA) and deep learning (i.e., long short-term memory (LSTM) model) for incorporating and utilizing the combined multi-temporal and spectral information from time series spectral imaging datasets. An example data, consisting of times series spectral images of casein-based biopolymers, was used to illustrate and evaluate the proposed hybrid approach. Compared to using partial least squares discriminant analysis (PLSDA), the proposed PCA-LSTM method applying the same spectral pretreatment achieved substantial improvement in the pixel-wise classification (i.e., accuracy increased from 59.97% of PLSDA to 85.73% of PCA-LSTM). When projecting the pixel-wise model to object-based classification, the PCA-LSTM approach produced an accuracy of 100%, correctly classifying the whole 21 film samples in the independent test set, while PLSDA only led to an accuracy of 80.95%. The proposed method is powerful and versatile in utilizing distinctive characteristics of time dependencies from multivariate time series dataset, which could be adapted to suit non-congruent images over time sequences as well as spectroscopic data. (C) 2020 The Authors. Published by Elsevier B.V.

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