4.7 Article

Robust ferromagnetism in wafer-scale monolayer and multilayer Fe3GeTe2

Journal

NPJ 2D MATERIALS AND APPLICATIONS
Volume 4, Issue 1, Pages -

Publisher

NATURE RESEARCH
DOI: 10.1038/s41699-020-00167-z

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Funding

  1. Max Planck-UBC-UTokyo Centre for Quantum Materials
  2. Canada First Research Excellence Fund, Quantum Materials and Future Technologies Program
  3. Natural Sciences and Engineering Research Council of Canada (NSERC)
  4. Canada Foundation for Innovation (CFI)

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Monolayer iron germanium telluride Fe3GeTe2, one of the typical two-dimensional ferromagnetic materials, hitherto, has only been studied by exfoliated micron-sized samples. We achieve high-quality wafer-scale growth of thin Fe(3)GeTe(2)films by molecular beam epitaxy, greatly expanding the types of characterization tools employable and providing the possibility for its integration in devices like consumer electronics. Thickness-dependent transport measurements are used to characterize and probe for magnetic order. Ferromagnetic states exist in 1-10 layer thick Fe3GeTe2, with Curie temperatures ranging from similar to 75 K in one layer samples to above 175 K in ten layer samples. A single ferromagnetic phase with significant magnetic anisotropy is revealed for all layer numbers. We submit the capability of synthesizing, wafer-scale Fe(3)GeTe(2)as an essential step towards its fulfillment in any applications involving magnetism, such as spintronics.

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