4.2 Article Proceedings Paper

Formation of orderedL1(0)-FePt phase in FePt-Ag thin films

Journal

APPLIED NANOSCIENCE
Volume 10, Issue 12, Pages 4809-4816

Publisher

SPRINGER HEIDELBERG
DOI: 10.1007/s13204-020-01552-2

Keywords

Stress state; Annealing; Ordering; L1(0)-FePt phase; Coercivity

Funding

  1. German Academic Exchange Service (DAAD) in the frame of the Leonard Euler scholarship program [57198300, 57291435]
  2. German Academic Exchange Service (DAAD) in the frame of the Visegrad Scholarship Program 2013/2014 (V4EaP Scholarship) [51300654]
  3. European Union [GINOP-2.3.2-15-2016-00041]
  4. European Regional Development Fund

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In this work, the influence of an Ag layer, which is located at different positions of the layer stack (top, intermediate, bottom), on the structural and magnetic properties of orderedL1(0)phase in Fe(50)Pt(50)films was investigated. It was found that the position of an additional Ag layer affects the stress state of the as-deposited FePt films. Mechanical stress is induced during deposition and post-annealing process due to the difference in thermal expansion coefficients and lattice mismatch of FePt, Ag, and substrate. The initial stress state affects the ordering process during subsequent heat treatment. The higher level of initial compressive stress (- 7.8 GPa) in FePt/Ag/FePt films results inL1(0)phase formation at a temperature of 700 degrees C which is about 100 degrees C lower than in films with Ag bottom (- 3.6 GPa) and top (+ 0.86 GPa) layers. A more pronounced (001) oriented growth of theL1(0)phase was observed in stacks with Ag top layer as compared to Ag bottom and intermediate layers. The highest values of coercivity were obtained for films with Ag intermediate and bottom layers, which is due to the distribution of Ag along FePt grain boundaries that result in strong exchange decoupling of FePt grains. Furthermore, the formation of the orderedL1(0)phase at comparatively low temperatures of about 370 degrees C was observed in a free-standing FePt/Ag (30 nm)/FePt film.

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