Graphdiyne as a saturable absorber for 2-μm all-solid-state Q-switched laser

As a novel one-atom-thick carbon allotrope, graphdiyne (GDY) has attracted wide interest in two-dimensional materials owing to its unique feature with a planar layer comprising sp(2)- and sp-hybridized carbon atoms and a direct natural bandgap. A high-quality saturable absorber (SA) based on GDY was successfully fabricated, and the nonlinear saturable absorption properties were investigated. A compact diode-pumped solid-state passively Q-switched laser based on the as-prepared GDY-SA could be operated at 2 mu m. The Q-switched laser delivered a maximum average output power of 1.29 W at a central wavelength of 1908.41 nm with up to 54.8% slope efficiency. A repetition rate of 91.58 kHz and single pulse energy of 23.08 mu J were obtained. This work is the first application of GDY as an SA to generate all-solid-state pulsed lasers. These results indicate that GDY is a promising SA for solid-state pulsed lasers and has further application potential for ultrafast photonic devices in the 2-mu m region.

Automated summary

Graphdiyne (GDY) as a novel one-atom-thick carbon allotrope has unique planar structure and direct natural bandgap, attracting wide interest in two-dimensional materials. A high-quality saturable absorber based on GDY was successfully applied in a compact diode-pumped solid-state passively Q-switched laser, achieving high output power and efficiency.