Journal
ADVANCED SCIENCE
Volume 7, Issue 22, Pages -Publisher
WILEY
DOI: 10.1002/advs.202002098
Keywords
high-energy detectors; metal halide perovskites; perovskite X-ray detectors; X-ray imagers; gamma-ray detectors
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Funding
- King Abdullah University of Science and Technology (KAUST) Office of Sponsored Research (OSR) [OSR-2018-CARF/CCF-3079.OSR-2018-CARF/CCF-3079]
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Metal halide perovskites (MHPs) have emerged as a frontrunner semiconductor technology for application in third generation photovoltaics while simultaneously making significant strides in other areas of optoelectronics. Photodetectors are one of the latest additions in an expanding list of applications of this fascinating family of materials. The extensive range of possible inorganic and hybrid perovskites coupled with their processing versatility and ability to convert external stimuli into easily measurable optical/electrical signals makes them an auspicious sensing element even for the high-energy domain of the electromagnetic spectrum. Key to this is the ability of MHPs to accommodate heavy elements while being able to form large, high-quality crystals and polycrystalline layers, making them one of the most promising emerging X-ray and gamma-ray detector technologies. Here, the fundamental principles of high-energy radiation detection are reviewed with emphasis on recent progress in the emerging and fascinating field of metal halide perovskite-based X-ray and gamma-ray detectors. The review starts with a discussion of the basic principles of high-energy radiation detection with focus on key performance metrics followed by a comprehensive summary of the recent progress in the field of perovskite-based detectors. The article concludes with a discussion of the remaining challenges and future perspectives.
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