Journal
ACS MACRO LETTERS
Volume 9, Issue 11, Pages 1527-1541Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsmacrolett.0c00629
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Funding
- National Research Foundation of Korea (NRF) - Korea government (MEST) [NRF-2017R1A2B3004763]
- Korea government (MSIT) [NRF 2017R1A5A1015365]
- Creative Materials Discovery Program through the NRF - Ministry of Science and ICT [2018M3D1A1058624]
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Scientific research on advanced polymer electrolytes has led to the emergence of all-solid-state energy storage/transfer systems. Early research began with acid-tethered polymers half a century ago, and research interest has gradually shifted to high-precision polymers with controllable acid functional groups and nanoscale morphologies. Consequently, various self-assembled acid-tethered block polymer morphologies have been produced. Their ion properties are profoundly affected by the multiscale intermolecular interactions in confinements. The creation of hierarchically organized ion/dipole arrangements inside the block copolymer nanostructures has been highlighted as a future method for developing advanced single-ion polymers with decoupled ion dynamics and polymer chain relaxation. Several emerging practical applications of the acid-tethered block copolymers have been explored to draw attention to the challenges and opportunities in developing state-of-the-art electrochemical systems.
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