Temporal Development of a Laser-Induced Helium Nanoplasma Measured through Auger Emission and Above-Threshold Ionization

Femtosecond pump-probe electron and ion spectroscopy is applied to study the development of a helium nanoplasma up to the nanosecond timescale. Electrons, bound by the deep confming mean-field potential, are elevated toward the vacuum level in the nanoplasma expansion. Subsequent electron recombination gives rise to transitions between He+ states, resulting in autoionization. The time-resolved analysis of the energy transfer to quasifree electrons reveals a transient depletion of the Auger emission, which allows for a temporal gate to map the distribution of delocalized electrons in the developing mean field. Furthermore, we trace the recombination of delocalized electrons near the vacuum level into highly excited Rydberg states. Transient above-threshold ionization is introduced as a diagnostic tool to resolve the dynamics. Thus, the development of the electron distribution in the nanoplasma mean-field potential can be monitored via the features observed in the emission spectra.