4.8 Article

Characteristic Timescales of the Local Moment Dynamics in Hund's Metals

Journal

PHYSICAL REVIEW LETTERS
Volume 125, Issue 8, Pages -

Publisher

AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.125.086402

Keywords

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Funding

  1. Austrian Science Fund (FWF) [SFB F41, I 2794-N35]
  2. Deutsche Forschungsgemeinschaft (DFG, German Research Foundation) [SFB 1170, 258499086, EXC 2147, 390858490]

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We study the characteristic timescales of the fluctuating local moments in Hund's metal systems for different degrees of correlation. By analyzing the dynamical spin susceptibility in the real-time domain, we determine the timescales controlling oscillation and damping of on-site fluctuations-a crucial factor for the detection of local moments with different experimental probes. We apply this procedure to different families of iron pnictides or chalcogenides, explaining the material trend in the discrepancies reported between experimental and theoretical estimates of their magnetic moments.

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