4.7 Article

Catalytic performance of a metal-free graphene oxide-Al2O3 composite assembled by 3D printing

Journal

JOURNAL OF THE EUROPEAN CERAMIC SOCIETY
Volume 41, Issue 2, Pages 1399-1406

Publisher

ELSEVIER SCI LTD
DOI: 10.1016/j.jeurceramsoc.2020.10.010

Keywords

3D printing; Graphene oxide-Al2O3 composites; Carbocatalysis; Graphene oxide; Heterogeneous catalysis

Funding

  1. Conselleria de Cultura, Educacion e Ordenacion Universitaria of the Galician Government [ED431B2017/70, ED431B 2019/43]
  2. Centro singular de Investigacion de Galicia accreditation 2016-2019 [ED431 G/09]
  3. Strategic Grouping AEMAT grant [ED431E2018/08]
  4. Spanish Ministry of Science, Innovation and Universities [MAT2017-90100-C2-1-P]

Ask authors/readers for more resources

This paper introduces a novel 3D printed metal-free graphene oxide-Al2O3 (GO-Al2O3) catalytic system, which combines the excellent catalytic effect and reaction scope of graphene oxide, the chemical stability and recyclability of the ceramic support, and the versatility and control over size of 3D printing technology, representing a significant step in the development of highly active, heterogeneous, and reusable ceramic catalysts.
This paper describes the first example of a 3D printed metal-free graphene oxide-Al2O3 (GO-Al2O3) catalytic system and evaluates its catalytic performance in model transformations. A new functional architecture creates synergies to combine the excellent catalytic effect and reaction scope of graphene oxide, the chemical stability and recyclability of the ceramic support, and the versatility and control over size of 3D printing technology. The graphene oxide-Al2O3 based catalyst presented here constitutes a step forward in the development of highly active, heterogeneous, and reusable ceramic catalysts.

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