Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 142, Issue 42, Pages 17908-17912Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.0c08450
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Funding
- TopSector HighTech Systems & Materials in the TKI project Early cancer diagnostics
- CNRS
- Agence Nationale de la Recherche [ANR-17-CE09-0034-01]
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Faradaic reactions at low supporting electrolyte concentrations induce convection via electroosmotic flows. Here we combine finite-element simulations and electrochemical measurements on microparticles at ultramicroelectrodes to explore this effect. We show that convection becomes the dominant form of mass transport for experiments at low salt concentrations, violating the common assumption that convection can be neglected.
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