Journal
JOURNAL OF ORGANIC CHEMISTRY
Volume 85, Issue 18, Pages 11989-11996Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.joc.0c01818
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Funding
- National Natural Science Foundation of China [21576296, 21776318, 21676302, 81703365]
- Fundamental Research Funds for Central South University [2019zzts222, 2020zzts401]
- Central South University
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Acyl oximes are directly used as the acyl radical precursors in the hydroacylation reactions for the first time. In this work, acyl radicals can be effectively generated via beta-scission of a phosphoranyl radical under photocatalytic conditions. As a result, the hydroacylation of alkenes triggered by the resulting acyl radicals leads to facile syntheses of a range of valuable ketones.
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