Journal
INORGANIC CHEMISTRY
Volume 59, Issue 17, Pages 12122-12131Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.0c01054
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Funding
- National Natural Science Foundation of China [21801170, 91833304]
- Shenzhen Science and Technology Program [KQTD20170330110107046]
- Science and Technology Innovation Commission of Shenzhen Municipality [JCYJ20190808172203553]
- China Postdoctoral Science Foundation [2019TQ0198]
- Natural Science Foundation of SZU [2019003]
- Department of Science and Technology of Guangdong Province [2019QN010617]
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Luminescent coinage metal complexes have shown promising applications as electrolurriinescent emitters, photocatalysts/photosensitizers, and bioimagingitlieranostic agents, rendering them attractive alternatives to transition metal complexes based on iridium, ruthenium, and platinum that have extremely low earth abundance. In comparison to the widely studied Au(I) and Cu(I) complexes, Ag(I) complexes have seldom been explored in this field because of their inferior emission properties. Herein, we report a novel series of [Ag(NAN)(pAp)]. xhrbitinghighlYefficientthermallYactivated delaed fluorescence busineasilYaccessible neutraldiamineyygs c hela t es.PF6cumPlexese pigandsandcoumerciaflyalailablealcillarV diPi 'Phte The Ph toinminescence-uantum yields (PLQYs) of the Ag(I) emitters ate< 62lndopeufilms.ThehlghpLQy-th a large delayed fluorescence ratio a to enabled the fabrication of s light-emittingorganic di des(oLEDs) with ahighmax'mumexternalguautum efficiency f8.76%'aongtheh'hest values for based superior e ssi nPr Peties and an excited staefetimelnrhenicr sec ndtegime, together with its potent itYtheseecteaAg(1) complex has' been sed for simh t e usceiIinagingandanticancer treatment in human liver carcinoma HepG2 cells) revealing theP tential fnescentAg(I) comPlexe'fnthiolog1calapPiicati'ns such as therancstics.
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