Journal
INORGANIC CHEMISTRY
Volume 59, Issue 22, Pages 16117-16121Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.inorgchem.0c01716
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Funding
- National Natural Science Foundation of China [21771074, 21103137]
- Northwest University [338050094]
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Two Dy-III complexes, [Dy(bbpen-F)X] [X = Cl (1), Br (2); H(2)bbpen-F = N,N'- bis(2-hydroxybenzyl)-N,N'- bis(5-fluoro-2-methylpyridyl)ethylenediamine], have been synthesized that show remarkable single-molecule-magnet behavior with effective barriers of magnetic reversal of 837.7 K for 1 and 1149.7 K for 2 under zero direct-current field and hysteresis loops up to 20 K for 1 and 30 K for 2, as confirmed by magnetic properties and ab initio calculations.
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