Journal
ENERGY & FUELS
Volume 34, Issue 9, Pages 11282-11289Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.energyfuels.0c02120
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Funding
- National Natural Science Foundation of China [51776206]
- Local Innovative and Research Teams Project of Guangdong Pearl River Talents Program [2017BT01N092]
- Postgraduate Research & Practice Innovation Program of Jiangsu Province [KYCX20_0095]
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The conversion of carbon dioxide (CO2) to value-added chemical compounds that can be used as precursors in many industrial processes is a very attractive approach to facilitate greenhouse gas reduction. Here, we demonstrated a high-efficiency bifunctional catalyst composed of sodium-modified Fe3O4 and hierarchical nanocrystalline HZSM-5 aggregates, which could prepare aromatics from CO2 with a high yield of 23.5% and CO2 conversion of 45.3% at the space velocity of 4000 mL/gcat/h. The results showed that the low proximity of the two components, a suitable mass ratio of iron/zeolite, and a high density of total acidity over the bifunctional catalyst are decisive factors for the high selectivity toward aromatics and high catalytic stability. This study provides a simple and efficient way for direct CO2 hydrogenation to aromatics.
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