Journal
APPLIED SURFACE SCIENCE
Volume 528, Issue -, Pages -Publisher
ELSEVIER
DOI: 10.1016/j.apsusc.2020.146928
Keywords
Porous graphene-like carbon hydrogel; Ag+; Adsorption; Organic dye
Categories
Funding
- National Natural Science Foundation of China [51674131, 21373005, 51902149]
- Natural Science Foundation of Liaoning Province of China [2019-MS-156, RC190346]
- Liaoning Revitalization Talents Program [XLYC1907197]
- Natural Science Foundation of Liaoning University [LDGY2019009, LDGY2019014]
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New strategies for adsorbing environmental pollutants such as Ag+ and organic dyes are still in urgent need. Based on this, we developed a highly efficient adsorbent, porous graphene-like carbon (PGC), by a simple cat- alysis process. A three dimensional porous graphene-like carbon hydrogel (3D-PGCH) was further obtained by introducing polyvinyl alcohol (PVA) and fully cross-linked via freeze-drying. The 3D-PGCH had a high adsorption capacity for Ag+ with an adsorption value of 234.32 mg g(-1) at pH 4 and 303 K. Its active ingredient PGC exhibited excellent adsorbing effect on methylene blue (MB), and the maximum adsorption was up to 13381.62 mg g(-1), about 32 times higher than that of using single PGC. Moreover, the adsorption-desorption experiment reflected a good recyclability of 3D-PGCH, whose adsorption capacity remained a high level after four cycle experiments. This study provides a positive choice for resource conservation and wastewater remediation.
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