Journal
ACS APPLIED MATERIALS & INTERFACES
Volume 12, Issue 39, Pages 43976-43983Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsami.0c12842
Keywords
organic single crystals; long-range ordering; ambipolar transport; organic light-emitting transistors; external quantum efficiencies
Funding
- National Natural Science Foundation of China [91833304, 21975078, 51703065]
- Natural Science Foundation of Guangdong Province [2019B030301003]
- Introduced Innovative R&D Team of Guangdong Province [201101C0105067115]
- 111 Project
- Fundamental Research Funds for the Central Universities
- Thousand Youth Talents Plan
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A cyano-substituted styrene derivative is synthesized and successfully prepared to lamellate single crystals through precisely controlling the crystal growth conditions. The lamellate single crystals with regular edge and smooth surface display intrinsically ordered stacking and high quality, all of which are of importance for high optoelectronic performance. The single-component light-emitting transistors based on the lamellate crystals offer striking device performance in terms of record external quantum efficiency of 2.02%, exceeding the benchmark value in this field. Such organic light-emitting single crystals provide a versatile platform for designing and engineering their structures and optoelectronic properties toward light-emitting devices.
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