Journal
COMPOSITES COMMUNICATIONS
Volume 20, Issue -, Pages -Publisher
ELSEVIER SCI LTD
DOI: 10.1016/j.coco.2020.04.010
Keywords
A-site cation deficiency; LaFeO3; Carbon nanosheet; Electromagnetic microwave absorption
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Funding
- Natural Science Foundation of Shandong Province [ZR2019YQ24]
- Qingchuang Talents Induction Program of Shandong Higher Education Institution (Research and Innovation Team of Structural-Functional Polymer Composites)
- National Natural Science Foundation of China [51407134, 51801001]
- China Postdoctoral Science Foundation [2016M590619, 2016M601878]
- Provincial Key Research and Development Program of Shaanxi [2019GY-197]
- Thousand Talents Plan
- WorldClass University and Discipline
- Taishan Scholar's Advantageous and Distinctive Discipline Program of Shandong Province
- World-Class Discipline Program of Shandong Province
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Wafer biscuit structure like hierarchical A-site cation deficiency perovskite at carbon and RGO hybrid composites-LaxFeO3-y/RGO are fabricated by a simple one-pot route. The quantitative ratios of A-site cation deficiency are designed, and was represented by x = 1.0, 0.8, 0.6, 0.4 and 0.2, respectively. Besides the morphology and phase structure, but the chemical composition, especially the O vacancy induced by the deficiency, was also studied by X-ray photoelectron spectroscopy (XPS) data. The electromagnetic microwave absorption capabilities of these composites were further studied. Accompanying with the appearance of A-site cation deficiency, the reflection loss (RL) was optimized instinctively. The minimum RL of La0.8FeO3-y/RGO reaches 36.23 dB with an effective band (RL <= 10dB) width of 3.92 GHz from 11.68 to 15.60 GHz at the matching thickness 2.00 mm, which was demonstrated the domain role of dielectric loss ascribed to the polarization of dipoles between O vacancy and Fe4+. When the deficiency increased, the band widths reached 4.72 GHz with the synergistic effect of magnetic and dielectric phase.
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