Journal
FRONTIERS IN MATERIALS
Volume 7, Issue -, Pages -Publisher
FRONTIERS MEDIA SA
DOI: 10.3389/fmats.2020.00111
Keywords
electrolytes; solid-state batteries (SSBs); challenges; perspectives; fundamental understanding
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Funding
- National Natural Science Foundation of China [51872209, 51972239]
- Zhejiang Provincial Natural Science Foundation of China [LZ17E020002]
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Compared with traditional lithium-ion systems, solid-state batteries could achieve high safety and energy density. Although great improvements have been made, especially in solid-state electrolytes, fundamental challenges still remain for the solid-state systems in terms of chemistry and mechanics. This review summarizes the fundamental issues in solid-state batteries with a focus on three critical phenomena: (i) the principles of developing high ionic conductors, (ii) structural evolution at chemically unstable electrolyte-electrode interfaces, and (iii) the effects of manufacturing solid-state batteries, including electrode, and electrolyte design. The future perspectives are also outlined to guide the development of solid-state batteries.
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