Journal
CHEM
Volume 6, Issue 6, Pages 1310-1326Publisher
CELL PRESS
DOI: 10.1016/j.chempr.2020.05.012
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Funding
- Natural Science Foundation of China [21801124]
- Air Force Office of Scientific Research [FA9550-18-1-0320]
- Shenzhen Science and Technology Innovation Committee [JCYJ20170817105905899, JCYJ20180504165709042]
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High-performance n-type (electron-transporting or n-channel) polymer semiconductors are critical components for the realization of various organic optoelectronic devices and complementary circuits, and recent progress has greatly advanced the performance of organic thin-film transistors, all-polymer solar cells, and organic thermoelectrics, to cite just a few. This Perspective focuses on the recent development of high-performance n-type polymer structures, particularly those based on the most investigated and novel electron-deficient building blocks, as well as summarizes the performance achieved in the above devices. In addition, this Perspective offers our insights into developing new electron-accepting building blocks and polymer design strategies, as well as discusses the challenges and opportunities in advancing n-type device performance.
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