Journal
CARBON LETTERS
Volume 31, Issue 1, Pages 107-115Publisher
SPRINGER JAPAN KK
DOI: 10.1007/s42823-020-00155-9
Keywords
Poly(3-dodecylthiophene); Carbon nanotube; Organic solar cell; Charge-carrier dynamics; Photophysics
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In this study, multi-walled carbon nanotube/poly(3-hexylthiophene) and CNT-graft-poly(3-dodecylthiophene)/P3HT nanohybrids were used in the active layers of polymer solar cells to investigate their effects on performance. It was found that the PSC composed of P3HT:PC71BM:CNT-graft-PDDT/P3HT exhibited the highest power conversion efficiency, with significantly increased Jsc and Voc.
Multi-walled carbon nanotube/poly(3-hexylthiophene) (CNT/P3HT) and CNT-graft-poly(3-dodecylthiophene) (PDDT)/P3HT nanohybrids were applied in active layers to study the effects of these nanostructures on the polymer solar cell (PSC) performance. The charge-carrier dynamics and photophysics were studied in the binary and ternary systems based on P3HT, pre-developed nanostructures and/or phenyl-C71-butyric acid methyl ester (PC71BM) through the electrochemical impedance spectroscopy and morphological analyses. The weaker bimolecular recombination in the photoactive layer, consisting of CNT-graft-PDDT/P3HT nanostructures, was confirmed by short-circuit current (J(sc)) and open-circuit voltage (V-oc) measurements as a function of light intensity. PSC composed of P3HT:PC71BM:CNT-graft-PDDT/P3HT PSC exhibited the highest PCE of 4.18% with significantly increased J(sc) and V-oc.
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