Journal
ACS PHOTONICS
Volume 7, Issue 8, Pages 2147-2152Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsphotonics.0c00614
Keywords
two-dimensional materials; spin properties; hexagonal boron nitride; boron vacancy centers
Categories
Funding
- Australian Research Council [DP180100077, DP190101058, DE180100810, CE200100010]
- Asian Office of Aerospace Research and Development [FA2386-20-1-4014]
- Australian Research Council [DE180100810] Funding Source: Australian Research Council
Ask authors/readers for more resources
Two-dimensional hexagonal boron nitride offers intriguing opportunities for advanced studies of light-matter interaction at the nanoscale, specifically for realizations in quantum nanophotonics. Here, we demonstrate the generation of optically addressable spin defects based on the negatively charged boron vacancy (V-B(-)) center. We show that these centers can be created in exfoliated hexagonal boron nitride using a variety of focused ion beams (nitrogen, xenon, and argon). Using a combination of laser and resonant microwave excitation, we carry out optically detected magnetic resonance spectroscopy measurements, which reveal a zero-field ground state splitting for the defect of similar to 3.46 GHz. We also perform photoluminescence excitation spectroscopy and temperature-dependent photoluminescence measurements to elucidate the photo-physical properties of the V-B(-) centers. Our results are important for advanced quantum and nanophotonics realizations involving manipulation and readout of spin defects in hexagonal boron nitride.
Authors
I am an author on this paper
Click your name to claim this paper and add it to your profile.
Reviews
Recommended
No Data Available