Journal
SPECTROCHIMICA ACTA PART A-MOLECULAR AND BIOMOLECULAR SPECTROSCOPY
Volume 243, Issue -, Pages -Publisher
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.saa.2020.118807
Keywords
Boron nitrogen co-doped carbon quantum dots; High fluorescence quantum yield; Static quenching; Inner filter effect; Cr(VI)
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Funding
- theNational Key Research and Development Programof China [2018YFD0701001]
- National Natural Science Foundation of China [31772073, 31671844]
- Key Research and Development Program of Jiangsu Province [BE2019359]
- Priority Academic Program Development of Jiangsu Higher Education Institutions (PAPD)
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A novel fluorescent probe based on the static quenching and the inner filter effect between boron nitrogen co-doped carbon quantum dots (B, N-CDs) and Cr(VI) was developed for the quantitative determination of Cr( VI) in real water samples. B, N-CDs were prepared using the hydrothermal method with ammonium citrate and bis(pinacolato) diboron as raw materials. Compared with undoped CDs, the fluorescence properties of the B, N-CDs were improved. The fluorescence quantum yield of the B, N-CDs was as high as 59.01%. After optimization of the experimental parameters, the B, N-CDs could be used as a fluorescence probe to detect Cr(VI). Strong linear correlation (R-2 = 0.9986) was established in the Cr(VI) concentration range 03-500 mu M. and a detection limit of 0.24 mu M was achieved. Moreover, the B, N-CDs successfully detected Cr(VI) in real water samples, indicating that they have broad application prospects in the sensitive detection of Cr(Vl). (C) 2020 Elsevier B.V. All rights reserved.
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