Journal
NATURE
Volume 583, Issue 7815, Pages 232-+Publisher
NATURE RESEARCH
DOI: 10.1038/s41586-020-2440-4
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Funding
- European Research Council (ERC) [639119]
- Deutsche Forschungsgemeinschaft [SFB-1073]
- European Research Council (ERC) [639119] Funding Source: European Research Council (ERC)
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Active optical control over matter is desirable in many scientific disciplines, with prominent examples in all-optical magnetic switching(1,2), light-induced metastable or exotic phases of solids(3-8) and the coherent control of chemical reactions(9,10). Typically, these approaches dynamically steer a system towards states or reaction products far from equilibrium. In solids, metal-to-insulator transitions are an important target for optical manipulation, offering ultrafast changes of the electronic(4) and lattice(11-16) properties. The impact of coherences on the efficiencies and thresholds of such transitions, however, remains a largely open subject. Here, we demonstrate coherent control over a metal-insulator structural phase transition in a quasi-one-dimensional solid-state surface system. A femtosecond double-pulse excitation scheme(17-20) is used to switch the system from the insulating to a metastable metallic state, and the corresponding structural changes are monitored by ultrafast low-energy electron diffraction(21,22). To govern the transition, we harness vibrational coherence in key structural modes connecting both phases, and observe delay-dependent oscillations in the double-pulse switching efficiency. Mode-selective coherent control of solids and surfaces could open new routesto switching chemical and physical functionalities, enabled by metastable and non-equilibrium states.
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