4.8 Article

Dynamic Exciton Funneling by Local Strain Control in a Monolayer Semiconductor

Journal

NANO LETTERS
Volume 20, Issue 9, Pages 6791-6797

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.0c02757

Keywords

2D materials; tungsten diselenide; local strain engineering; exciton funneling

Funding

  1. Army Research Office (ARO) Multidisciplinary University Research Initiative (MUM) program [W911NF-18-1-0431]
  2. National Science Foundation (NSF) Research Advanced by Interdisciplinary Science and Engineering (RAISE) [CHE-1839155]
  3. National Science Foundation EFRI 2-DARE [1542863]
  4. CREST, JST [JPMJCR15F3]
  5. Samsung Scholarship
  6. Elemental Strategy Initiative by MEXT, Japan

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The ability to control excitons in semiconductors underlies numerous proposed applications, from excitonic circuits to energy transport. Two dimensional (2D) semiconductors are particularly promising for room-temperature applications due to their large exciton binding energy and enormous stretchability. Although the strain-induced static exciton flux has been observed in predetermined structures, dynamic control of exciton flux represents an outstanding challenge. Here, we introduce a method to tune the bandgap of suspended 2D semiconductors by applying a local strain gradient with a nanoscale tip. This strain allows us to locally and reversibly shift the exciton energy and to steer the exciton flux over micrometer-scale distances. We anticipate that our result not only marks an important experimental tool but will also open a broad range of new applications from information processing to energy conversion.

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