4.8 Article

Raman Scattering Cross Section of Confined Carbyne

Journal

NANO LETTERS
Volume 20, Issue 9, Pages 6750-6755

Publisher

AMER CHEMICAL SOC
DOI: 10.1021/acs.nanolett.0c02632

Keywords

carbyne; linear carbon chains; Raman scattering; Raman scattering cross section; TERS

Funding

  1. Swiss National Science Foundation [200020_192362/1]
  2. ETH Research [ETH-15 19-1]
  3. ETH Zurich Career Seed Grant [SEED -16 17-1]
  4. National Natural Science Foundation of China [51902353]
  5. Natural Science Foundation of Guangdong Province [2019A1515011227]
  6. FWF [P27769 -N20]
  7. Swiss National Science Foundation (SNF) [200020_192362] Funding Source: Swiss National Science Foundation (SNF)

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We experimentally quantify the Raman scattering from individual carbyne chains confined in double-walled carbon nanotubes. We find that the resonant differential Raman cross section of confined carbyne is on the order of 10(-22) cm(2) sr(-1) per atom, making it the strongest Raman scatterer ever reported.

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