Journal
MATERIALS CHEMISTRY AND PHYSICS
Volume 248, Issue -, Pages -Publisher
ELSEVIER SCIENCE SA
DOI: 10.1016/j.matchemphys.2020.122873
Keywords
CNTs-Ag-TiO2 ternary structure; Photocatalysis; Visible light; Degradation mechanism
Categories
Funding
- National Natural Science Foundation of China of China [11204082]
- Shanghai Natural Fund [16ZR1410700]
- Fundamental Research Funds for the Central Universities
- Project of Social Office of Shanghai Science and Technology Commission [19DZ1205102]
- [201902 ZR]
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In order to improve the catalytic efficiency of titanium dioxide (TiO2) under visible light, TiO2 nanoparticles was composed with the silver-covered carbon nanotubes (CA) to form CNTs-Ag-TiO2 (CAT) ternary structure via in situ reduction combined with sol-gel method. The composite was characterized by X-ray diffraction (XRD), scanning electron microscopy (SEM), X-ray photoelectron spectroscopy (XPS), diffuse reflectance spectra (DRS) and photoluminescence (PL) spectra. Using methylene blue (MB) as the model pollutant, photocatalytic activity of CAT was studied to investigate the influence of the composited amount of CA on the effect of photocatalysis. The results revealed that the photocatalytic activity of TiO2 under both visible light and UV light were improved by compositing with CA. When the mass ratio of CA is 15%, the degradation rare of methylene blue (MB) by CAT reached to 80.8% under visible light in 3 h, which is 16.5 times higher than that of TiO2. Accordingly, the degradation rate reached to 99.2% under UV light in 40 min, which is nearly twice as fast as that of TiO2.
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