Journal
JOURNAL OF POROUS MATERIALS
Volume 27, Issue 6, Pages 1765-1771Publisher
SPRINGER
DOI: 10.1007/s10934-020-00952-7
Keywords
Poly(2; 6-diaminopyridine); Honeycomb-like structure; N-doped carbon; Supercapacitors
Funding
- National Natural Science Foundation of China [517720835, 51472083]
- Hunan Provincial Natural Science Foundation of China [2017JJ2008]
- Science and Technology Planning Project of Hunan Province [2018GK1030]
- Growth Scheme for Young Teachers of Hunan University [531107040185]
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Honeycomb-like nitrogen-doped porous carbon (HNC) is prepared by using poly(2,6-diaminopyridine) as nitrogen-enriched precursor and silica as hard template. After carbonization and template removal, the obtained HNC possesses an interconnected 3D hierarchical porous structure and a nitrogen level up to 15.31 at.%. Owing to the hierarchical porous structure and abundant active sites in the carbon matrix, the HNC exhibits an excellent capacitive performance with a high specific capacitance of 398 F g(-1)at a current density of 0.1 A g(-1)and exceptional cycling stability (110.4% retention after 5000 cycles). This work provides a facile and efficient strategy for the large-scale production of nitrogen superdoped interconnected hierarchical carbon framework for high performance supercapacitors.
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