Journal
CHINESE JOURNAL OF CHEMISTRY
Volume 38, Issue 10, Pages 1132-1152Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cjoc.202000270
Keywords
Cyclization; Cycloaddition; Aryl diazonium salts; N-Heterocycles; Synthesis
Categories
Funding
- National Key Research and Development Program of China [2019YFA0905100]
- National Natural Science Foundation of China [21772142, 21901181, 21971186]
- Tianjin Municipal Science & Technology Commission [19JCQNJC04700]
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Aryl diazonium salts occupy a privileged role in synthetic chemistry owing to their ready availability and versatile reactivity. While their applications in accessing diversely functionalized arene derivatives via denitrogenation-coupling and reduction/addition reactions have been well recognized by practitioners in both academia and industry, recent renaissance in chemical transformations of retaining the key N-2-unit has emerged as a powerful technique to construct variousN-heterocycles. This review covers the history and latest advances in cyclization and cycloaddition reactions using aryl diazonium salts as N-2-annulation synthons. The scope, applications, and opportunities in exploring new chemical space by this sustainable strategy are summarized and discussed.
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