Journal
CHINESE CHEMICAL LETTERS
Volume 32, Issue 2, Pages 649-659Publisher
ELSEVIER SCIENCE INC
DOI: 10.1016/j.cclet.2020.07.040
Keywords
Metal-organic framework composites; CO2 chemical fixation; CO2 hydrogenation; CO2 photoreduction; CO2 electroreduction; CO2 photoelectroreduction
Categories
Funding
- National Natural Science Foundation of China [21773314, 21720102007, 21821003, 21890382]
- Guangdong Natural Science Funds for Distinguished Young Scholar [2019B151502017]
- Tip-top Youth Talents of Guangdong special support program [20173100042150021]
- Science and Technology Planning Project of Guangzhou [201707010168]
- China Postdoctoral Science Foundation [2019M662809]
- Local Innovative and Research Teams Project of Guangdong Peal River Talents Program [2017BT01C161]
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This review focuses on the synthesis and catalytic applications of metal-organic framework (MOF) composites for CO2 capture and conversion (C3), covering synthetic strategies, recent progress, and challenges and future prospects in the field.
Reliable technologies for CO2 capture and conversion (C3) are of vital importance for the establishment of a sustainable society. Metal-organic framework (MOF) composites have shown their compelling potentials for C3 due to the plentiful reticular chemistry of MOF structures and the synergistic catalysis between MOFs and the functional guests. This review focuses on the syntheses and catalytic applications towards C3 of MOF composites, which is divided into three sections. The first section gives a brief introduction about synthetic strategies of MOF composites. The second section discusses the recent progress of MOF composites in C3, including CO2 chemical fixation, hydrogenation, photoreduction, electroreduction and photoelectroreduction. The third section summarizes the challenges and future prospects of MOF composites for C3. We hope that this review cannot only provide an inspiration for the rational design of MOF composites for C3, but also stimulate more and more research works in this emerging area. (C) 2020 Chinese Chemical Society and Institute of Materia Medica, Chinese Academy of Medical Sciences. Published by Elsevier B.V. All rights reserved.
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