4.7 Review

Recent progress on photocatalytic heterostructures with full solar spectral responses

Journal

CHEMICAL ENGINEERING JOURNAL
Volume 393, Issue -, Pages -

Publisher

ELSEVIER SCIENCE SA
DOI: 10.1016/j.cej.2020.124719

Keywords

Heterostructures; Near infrared (NIR) light; Full solar-light response; Photocatalytic mechanism; Environmental and energy applications

Funding

  1. Natural Science Foundation of Hunan Province [2019JJ50127]
  2. General Project of Hunan Education Department [19C0538, 18A273]
  3. Provincial Natural Science Foundation
  4. Natural Science Foundation of Jiangsu Province [BK20160383]
  5. Wuhan University

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Photocatalysis has received significant attention as a technology that can solve global energy and environmental issues that are essential for the sustainable development of society. The use of solar light and separated photo-generated charges plays an important role in enhancing photocatalytic efficiency. Constructing heterostructure-based full-solar-light-driven photocatalysts is a sensible method for widening the solar light response and accelerating charge migration. This review comprehensively summarizes progress in heterostructure development for use in full-solar-light-driven photocatalytic systems, including basic photo-response theory, photocatalytic mechanisms, and applications including environmental decontamination, water-splitting, CO2 conversion, and photocatalytic oxidation reactions. This review provides an in-depth discussion regarding the fundamental principles associated with solar-light harvesting and efficient charge migration that are crucial for heterostructure design. Therefore, this review provides inspiration for the development of further innovations in the full-solar-light-driven photocatalysis field.

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