Journal
ANGEWANDTE CHEMIE-INTERNATIONAL EDITION
Volume 59, Issue 42, Pages 18405-18411Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/anie.202006793
Keywords
nanocapsules; organized media; RAFT polymerization
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Funding
- National Science Foundation [CHE-1709921]
- University of Connecticut Research Excellence Program
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Co-localization of monomers, crosslinkers, and chain-transfer agents (CTA) within self-assembled bilayers in an aqueous suspension enabled the successful directed assembly of nanocapsules using a reversible addition-fragmentation chain transfer (RAFT) process without compromising the polymerization kinetics. This study uncovered substantial influence of the organized medium on the course of the reaction, including differential reactivity based on placement and mobility of monomers, crosslinkers, and CTAs within the bilayer.
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