Journal
CHINESE JOURNAL OF CHEMISTRY
Volume 34, Issue 12, Pages 1225-1235Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/cjoc.201600592
Keywords
alkylation of aldehyde; chiral-at-metal complex; synergistic catalysis
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Funding
- National Natural Science Foundation of China [21302183]
- Strategic Priority Research Program of the Chinese Academy of Sciences [XDA09030102]
- 100 Talents Programme of the Chinese Academy of Sciences
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A synergistic catalysis combination of chiral-at-metal rhodium complex and amine catalyst was developed for enantioselective alkylation of aldehydes with alpha,beta-unsaturated 2-acyl imidazoles. The corresponding adducts were obtained in good yields with excellent enantioselectivities (up to 99% ee).
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