Journal
ADVANCED MATERIALS
Volume 32, Issue 37, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202002748
Keywords
bioelectronics; ethylene-glycol-functionalized polymers; mixed ionic-electronic conduction; organic electrochemical transistors
Categories
Funding
- KAUST
- King Abdullah University of Science and Technology Office of Sponsored Research (OSR) [OSR-2018-CARF/CCF-3079, OSR-2015-CRG4-2572, OSR-4106 CPF2019]
- EC FP7 Project SC2 [610115]
- EC H2020 [643791]
- EPSRC [EP/G037515/1, EP/M005143/1, EP/L016702/1]
- Knut and Alice Wallenberg Foundation
- Wallenberg Wood Science Center [KAW 2018.0452]
- Swedish Government Strategic Research Area in Materials Science on Advanced Functional Materials at Linkoping University [2009-00971]
- TomKat Center for Sustainable Energy at Stanford University
- EPSRC [EP/M005143/1] Funding Source: UKRI
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A series of glycolated polythiophenes for use in organic electrochemical transistors (OECTs) is designed and synthesized, differing in the distribution of their ethylene glycol chains that are tethered to the conjugated backbone. While side chain redistribution does not have a significant impact on the optoelectronic properties of the polymers, this molecular engineering strategy strongly impacts the water uptake achieved in the polymers. By careful optimization of the water uptake in the polymer films, OECTs with unprecedented steady-state performances in terms of [mu C*] and current retentions up to 98% over 700 electrochemical switching cycles are developed.
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