Journal
ADVANCED MATERIALS
Volume 32, Issue 28, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adma.202001227
Keywords
biomaterial devices; light-stimulated synaptic transistors; multifunctional devices; organic field-effect transistors; photodetectors
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Funding
- National Natural Science Foundation of China [61822405]
- Science & Technology Foundation of Shanghai [19JC1412402]
- Shanghai Education Development Foundation
- Shanghai Municipal Education Commission [18SG20]
- National Key Research and Development Program of China [2017YFA0103904]
- Ministry of Science and Technology of China [2018YFA0703200]
- Fundamental Research Funds for the Central Universities
- Shuguang Program
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Inspired by the photosynthesis process of natural plants, multifunctional transistors based on natural biomaterial chlorophyll and organic semiconductors (OSCs) are reported. Functions as photodetectors (PDs) and light-stimulated synaptic transistors (LSSTs) can be switched by gate voltage. As PDs, the devices exhibit ultrahigh photoresponsivity up to 2 x 10(6) A W-1, detectivity of 6 x 10(15) Jones, and I-photo/I-dark ratio of 2.7 x 10(6), which make them among the best reported organic PDs. As LSSTs, important synaptic functions similar to biological synapses are demonstrated, together with a dynamic learning and forgetting process and image-processing function. Significantly, benefiting from the ultrahigh photosensitivity of chlorophyll, the lowest operating voltage and energy consumption of the LSSTs can be 10(-5) V and 0.25 fJ, respectively. The devices also exhibit high flexibility and long-term air stability. This work provides a new guide for developing organic electronics based on natural biomaterials.
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