Journal
ADVANCED FUNCTIONAL MATERIALS
Volume 30, Issue 30, Pages -Publisher
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adfm.202002021
Keywords
black phosphorus; carbon nitride; photocatalysis; water splitting
Categories
Funding
- National Natural Science Foundation of China [21902051, 21761132002, 21861130353, U1905214, 21961142019]
- Natural Science Foundation of Fujian Province [2019J05090, 2017J01014]
- Graphene Power and Composite Research Center of Fujian Province [2017H2001]
- Scientific Research Funds of Huaqiao University [605-50Y17060]
- Open Project Program of the State Key Laboratory of Photocatalysis on Energy and Environment of Fuzhou University [SKLPEE-201803]
- National Key Technologies RAMP
- D Program of China [2018YFA0209301]
- National Basic Research Program of China [2013CB632405]
- Chang Jiang Scholars Program of China [T2016147]
- 111 Project [D16008]
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The development of metal-free photocatalysts with high efficiency, stability, and broadband solar absorption is a major challenge to realize green and sustainable chemical development. Recently, metal-free nanohybrids (BP/CN) composed of black phosphorus (BP) and polymeric carbon nitride (CN) are emerged as photocatalytic hybrids with broadband light-harvesting capabilities and higher photocatalytic performance. Herein, the latest progress of BP/CN hybrids for multifarious photoredox reactions is summarized. The different heterojunction types of BP/CN hybrid photocatalysts, including type I, type II, and multicomponent heterojunctions, are illustrated. Furthermore, the relevant applications of BP/CN hybrid photocatalysts for photocatalytic water splitting, CO2 photoreduction, N-2 fixation, H2O2 production, pollutant decomposition, and bacterial inactivation are discussed. An overview of the challenge in this area and the directions for the future is presented.
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