Journal
ACS NANO
Volume 14, Issue 10, Pages 12895-12904Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsnano.0c03849
Keywords
Laplace pressure imbalance; droplet self-propulsion; nano/microtexturing; superhydrophobicity; laser micromachining; droplet merging; drop impact
Categories
Funding
- European Union [801229]
- Commission for Technology and Innovation (CTI) under the Swiss Competence Centers for Energy Research -Efficiency of Industrial Processes (SCCER-EIP) program [KTI.2014.0148]
- Swiss National Science Foundation (SNF) [169654]
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Liquid transport (continuous or segmented) in microfluidic platforms typically pumping devices or external fields working collaboratively with special Hula. properties to enable fluid motion. Natural liquid adhesion on surfaces deters motion land promotes the possibility of liquid or surface contamination. Despite progress, significant advancements are needed before devices for passive liquid Propulsion, without the input of external energy and unwanted contamination, become a reality in applications. Here we present an unexplored and facile approach based on the Laplace pressure imbalance, manifesting itself through l targeted track texturing, driving passively droplet motion, while maintaining the limited of the Cassie-Baxter state on superhydrophobic surfaces. The track topography resembles out-of-plane, backgammon-board, slowly converging microridges decorated with nanotexturing. This design naturally deforms lasymmetrically the menisci formed at the bottom of la droplet contacting such tracks and causes a Laplace pressure imbalance that drives droplet motion. We investigate this effect over a range of opening track angles and develop a model to explain and quantify the underlying mueichiac platform'of droplet self-propulsion. We further implement the developed topography for applications relevant to microfld functionalities. We demonstrate control lof the rebound angle of vertically impactingdroplets, achieve horizontal self-transport to distances up to 65 times the droplet diameter, show significant uphill motion against gravity, and illustrate a self-driven droplet-merging process.
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