Journal
PHYSICAL REVIEW MATERIALS
Volume 4, Issue 6, Pages -Publisher
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevMaterials.4.064201
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Funding
- National Key Research and Development Program of China [2017YFA0303603, 2016YFA0300303, 2016YFA0300604]
- National Natural Science Foundation of China [11774408, 11574383, 11874417]
- Strategic Priority Research Program of CAS [XDB30000000]
- International Partnership Program of Chinese Academy of Sciences [GJHZ1826]
- Beijing Natural Science Foundation [4191003]
- CAS Interdisciplinary Innovation Team
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We report ultrafast quasiparticle (QP) dynamics of TaAs, from which we obtain its electron-phonon coupling (EPC) strength. Two relaxation components with lifetimes tau(f)(ast) = 0.48 ps and tau(slow) = 250 ps are observed, each of which exhibits a smooth temperature dependence. Furthermore, we carry out a fluence-dependence investigation, based on which the quantitative analysis of the fast relaxation component yields a constant EPC strength lambda with lambda /(2) approximate to 5.2 ps(-1). In addition, our rotational polarization angle experiment demonstrates that the QP ultrafast dynamics is nearly isotropic under the given excitation geometry. Our investigation of the EPC strength accounts for the so far relatively rarely explored medium fluence regime, which can be generalized to various types of quantum materials.
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