Journal
JOURNAL OF ENERGY CHEMISTRY
Volume 53, Issue -, Pages 208-225Publisher
ELSEVIER
DOI: 10.1016/j.jechem.2020.04.063
Keywords
Defect; Electrocatalysts; Vacancies; Heteroatom doping
Funding
- National Natural Science Foundation of China [21573066, 21825201, 2187350, 51402100, 21905088]
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This review summarizes recent progress in defect electrocatalysts, highlighting the importance of dynamic evolution of defect sites for designing and preparing high-performance electrocatalysts. Furthermore, it suggests future possibilities for the reasonable design of defect electrocatalysts to obtain desirable performance due to insufficient understanding of the defect-structure-property relationships.
This review briefly summarizes recent progress in defect electrocatalysts, and the synthesis strategies and characterization techniques for defects are systematically discussed. Although challenges in the characterization of defect structures in the electrocatalytic reaction process remain, the dynamic evolution of defect sites is predicted to be helpful for designing and preparing high-performance electrocatalysts for commercial applications. Furthermore, due to an insufficient understanding of the defect-structure-property relationships, future possibilities for the reasonable design of defect electrocatalysts to obtain desirable performance are suggested. (C) 2020 Science Press and Dalian Institute of Chemical Physics, Chinese Academy of Sciences. Published by ELSEVIER B.V. and Science Press. All rights reserved.
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