Journal
ACS MACRO LETTERS
Volume 9, Issue 4, Pages 454-458Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acsmacrolett.0c00090
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Funding
- National Natural Science Foundation of China [21971179, 21774083]
- Priority Academic Program Development of Jiangsu Higher Education Institutions
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Scalable synthesis of multicompartment polyion complex (PIC) systems has been achieved via visible light-initiated RAFT polymerization of cationic monomer in the presence of anionic diblock copolymer micelles in water at 25 degrees C. This polymerization-induced hierarchical electrostatic self-assembly (hierarchical PIESA) implements structural hierarchy via programmable self-assembly to form multicompartment PIC micelles and their monolayer colloidal nanosheets and nanocages. The anionic micelles play decisive roles in such a hierarchical PIESA to access biologically relevant yet otherwise inaccessible multicompartment PIC systems.
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