Journal
SYNLETT
Volume 31, Issue 11, Pages 1077-1082Publisher
GEORG THIEME VERLAG KG
DOI: 10.1055/s-0040-1707121
Keywords
asymmetric synthesis; copper-catalyzed; N; -monoarylation; sulfonamide; diaryliodonium salt; desymmetrization
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Funding
- National Natural Science Foundation of China [21602095]
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A copper-catalyzed asymmetric intermolecular N -monoarylation of weakly nucleophilic sulfonamide by desymmetrization of cyclic diaryliodonium salts has been developed. Chiral copper(II)-diamine ligand complexes catalyzed this intermolecular asymmetric aryl C-N cross-coupling reaction effectively at room temperature to afford a series of N -monoarylsulfonamides in good to excellent yields and enantioselectivities.
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