Journal
CHEMISTRY OF MATERIALS
Volume 28, Issue 4, Pages 1213-1219Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.chemmater.5b04887
Keywords
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Funding
- Inorganometallic Catalyst Design Center, an Energy Frontier Research Center - U.S. Department of Energy, Office of Science, Basic Energy Sciences [DE-SC0012702]
- MRSEC program at the Materials Research Center [NSF DMR-1121262]
- International Institute for Nanotechnology (IIN)
- State of Illinois, through the IIN
- MRSEC program of the National Science Foundation at the Materials Research Center of Northwestern University [DMR-1121262]
- International Institute for Nanotechnology
- MRSEC [NSF DMR-1121262]
- Keck Foundation
- State of Illinois
- Northwestern University
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The combination (AIM-ME) of atomic layer deposition in metal organic frameworks (MOFs) and metal exchange (ME) is introduced as a technique to install dispersed metal atoms into the mesoporous MOF, NU-1000. Zn-AIM, which contains four Zn atoms per Zr-6 node, has been synthesized through AIM and further characterized through density functional calculations to provide insight into the possible structure. Zn-AIM was then subjected to modification via transmetalation to yield uniform porous materials that present nonstructural Cu, Co, or Ni atoms.
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