Journal
SCIENCE CHINA-CHEMISTRY
Volume 63, Issue 5, Pages 692-698Publisher
SCIENCE PRESS
DOI: 10.1007/s11426-019-9711-x
Keywords
multi-layer 3D chirality; organo sandwich chirality; architecture chirality; aggregation-induced emission (AIE); charge transfer (CT)
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Funding
- National Natural Science Foundation of China [91956110, 21672100]
- Robert A. Welch Foundation (USA) [D-1361]
- Beijing National Laboratory for Molecular Sciences [BNLMS201910]
- School of Pharmaceutical Science and Technology (SPST), Tianjin University, Tianjin, China
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New synthesis of multi-layer 3D chiral molecules has been developed under novel conditions to give better outcomes. The aggregation-induced emission (AIE), UV irradiation/excitation, charge transfer (CT) and local excited (LE) pi pi* transitions have been investigated on a representative individual enantiomer of pseudo C-2 asymmetry which was made possibly by differentiating moieties on phosphorous on N-phosphonyl ring of chiral sandwich framework. Meanwhile, a new tandem C-N/C-C coupling reaction was unexpectedly rendered providing a novel access to special benzo[a]carbazoles.
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