Journal
PETROLEUM SCIENCE AND TECHNOLOGY
Volume 38, Issue 6, Pages 618-625Publisher
TAYLOR & FRANCIS INC
DOI: 10.1080/10916466.2020.1774605
Keywords
Bimetallic catalysts; CeO2 support; hydrogen production; steam reforming
Funding
- China Postdoctoral Science Foundation [2019M651094]
- National Natural Science Foundation of China [51779025]
- Natural Science Foundation of Liaoning Province [2019-ZD-0154]
- Fundamental Research Funds for the Central Universities of China [3132019327]
- Innovation and Startup Business Education Project of Universities in Guangzhou [2019PT201]
- Innovative strong School Project of Guangzhou Maritime University [F410102]
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Methane steam reforming (MSR) reaction is a promising industrial hydrogen production technology. In this study, the impregnation method was deployed to prepare mono Co and Co-based bimetallic catalysts loaded on CeO(2)nanoparticles as the catalysts for MSR. Results show that the improved Co-based bimetallic catalysts have good performance compared to the mono one. The best catalyst sample was Co-Ni/CeO(2)which resulted in the CH(4)conversion of 76.1%, H(2)selectivity of 58.5% and H(2)yield of 44.5%. Furthermore, the H(2)selectivity increased significantly from 58.5% to 77.2% with the increase of the total Co-Ni metal loading amount.
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