Journal
ORGANIC LETTERS
Volume 22, Issue 11, Pages 4196-4200Publisher
AMER CHEMICAL SOC
DOI: 10.1021/acs.orglett.0c01259
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Funding
- UIC Department of Chemistry
- National Science Foundation (CAREER Award) [1654490]
- UIC Chancellors Undergraduate Research Award
- Division Of Chemistry
- Direct For Mathematical & Physical Scien [1654490] Funding Source: National Science Foundation
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A novel non-aromatic pool synthetic strategy for the synthesis of benzofuran-based natural products via oxidative haloaromatization of enones is reported. This approach is successfully applied in the first total synthesis of the natural product aspergillusene B. In comparison with a separately executed aromatic pool synthesis, the non-aromatic pool protocol demonstrates equivalent efficiency but offers a much higher degree of modularity.
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