Journal
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
Volume 142, Issue 19, Pages 8755-8762Publisher
AMER CHEMICAL SOC
DOI: 10.1021/jacs.0c01023
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Funding
- National Natural Science Foundation of China [51702365]
- Key Research and Development Plan of Shandong Province [2019GGX102056, 2018GGX104018]
- Special Project Fund of Taishan Scholars of Shandong Province [ts201511017]
- Fundamental Research Funds for the Central Universities [16CX05006A, 19CX05002A]
- New Faculty Start-up funding in China University of Petroleum (East China) [YJ201501029]
- Australian Research Council (ARC) [DE190101410, FT150100479]
- Australian Research Council [DE190101410] Funding Source: Australian Research Council
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The assembly of two-dimensional (2D) nanosheets into three-dimensional (3D) well-organized superstructures is one of the key topics in materials chemistry and physics, due to their potential applications in various fields. Herein, starting from the crystalline metal-organic framework (MOF) particles, a spherical superstructure consisting of metal-organic framework nanosheets (SS-MOFNSs) is synthesized via a simple solvothermal transformation process. After pyrolysis and nitrogenization in ammonia, the SS-MOFNSs are further transformed into the spherical superstructure consisting of boron nitride nanosheets (SS-BNNSs), which preserve the original spherical superstructure morphology. Taking advantage of this unique superstructure, the resulting SS-BNNSs exhibit excellent catalytic activity for selective oxidative dehydrogenation of propane to produce propylene and ethylene. The results of this work provide a novel synthetic strategy to fabricate 3D spherical superstructures consisting of 2D nanosheets for high-performance applications in catalysis, energy storage, as well as other related fields.
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