Journal
JOURNAL OF POLYMER RESEARCH
Volume 27, Issue 6, Pages -Publisher
SPRINGER
DOI: 10.1007/s10965-020-02152-y
Keywords
Polyimide fiber; Bisphenol A dicyanate esters resin; Composite laminates; Dielectric properties; Mechanical properties
Categories
Funding
- National Key Research and Development Program of China [2017YFB0308103]
- National Natural Science Foundation of China [51773007]
- Science and Technology on Transient Impact Laboratory Foundation [6142606183208]
- Fundamental Research Funds for the Central Universities [XK1802-2]
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Polyimide (PI)/ bisphenol A dicyanate esters (BADCy) composite laminates with varying resin contents were prepared by filament winding and autoclave molding process. The laminates exhibited ultralow dielectric constant (epsilon of 3.15-3.25) and dielectric loss (tan delta of 0.004-0.006) as well as excellent mechanical properties. When the resin content was 35.6%, the composite achieved outstanding comprehensive properties with tensile strength and modulus equal to 1485.1 MPa and 80.9 GPa, respectively, and the inter-laminar shear strength (ILSS) up to 66.2 MPa. The failure mode of laminates followed an explosive gage middle (XGM) mechanism, which suggested a favorable interface between fiber and resin. According to the mixed law equation, PI fiber at a frequency of 10.2 GHz exhibited dielectric constant of 3.41 +/- 0.03 and dielectric loss of about 0.002-0.004. The successful preparation of PI fiber reinforced BADCy composite with low dielectric constant provides new ideas for material design and selection of lightweight high-strength structural-functional integrated composites.
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