Journal
CHEMICAL COMMUNICATIONS
Volume 52, Issue 12, Pages 2497-2500Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc08741d
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Funding
- CTI Swiss Competence Center of Energy Research (SCCER) on Heat and Electricity Storage
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The catalytic N-formylation and N-methylation of amines using CO2 as the carbon source represents a facile and sustainable approach for the synthesis of pharmaceuticals and natural products. Herein, we describe highly effective and inexpensive thiazolium carbene-based catalysts derived from vitamin B1 for the N-formylation and N-methylation of amines, using polymethylhydrosiloxane (PMHS) as a reducing agent, which operate under ambient conditions.
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