Journal
CHEMICAL COMMUNICATIONS
Volume 52, Issue 10, Pages 2027-2030Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c5cc09446a
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Funding
- SERB, India [EMR/2014/000164]
- UGC India
- IIT-B
- CSIR India
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Tremendous progress has been made towards ortho-selective C-H functionalization in the last three decades. However, the activation of distal C-H bonds and their functionalization has remained fairly underdeveloped. Herein, we report sequential meta-C-H functionalization by performing selective mono-olefination and bis-olefination with late stage modification of the C-Si as well as Si-O bonds. Temporary silyl connection was found to be advantageous due to its easy installation, easy removal and wide synthetic diversification.
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