Journal
CHEMICAL COMMUNICATIONS
Volume 52, Issue 36, Pages 6091-6094Publisher
ROYAL SOC CHEMISTRY
DOI: 10.1039/c6cc02131j
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Funding
- NSFC [21231005, 21322101]
- MOE [B12015, IRT13R30]
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A solid lithium superionic conductor Li11AlP2S12 with a thio-LISICON analogous structure has been synthesized for the first time by sintering at 500 degrees C (LAlPS500). Such a pure lithium ionic conductor shows a conductivity of 8.02 x 10(-4) S cm(-1) at 25 degrees C, a low E-a of 25.4 kJmol(-1), and a wide electrochemical voltage window of higher than 5.0 V (vs. Li+/Li). This facilitation of Li ionic conduction suggests the potential application in solid lithium ion batteries.
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